By Yun Hang Hu
content material: CONTENTS; PREFACE; 1. SYNTHESIS AND CHARACTERIZATION OF FERRITE fabrics FOR THERMOCHEMICAL CO2 SPLITTING utilizing focused solar power; ANDREA AMBROSINI, ERIC N. COKER, MARK A. RODRIGUEZ, STEPHANIE LIVERS, LINDSEY R. EVANS, JAMES E. MILLER, AND ELLEN B. STECHEL; 2. PHOTOCATALYTIC relief OF CO2 utilizing H2 AS REDUCTANT OVER reliable BASE PHOTOCATALYSTS; KENTARO TERAMURA AND TSUNEHIRO TANAKA; three. CO2 SPLITTING through THE sun THERMOCHEMICAL CYCLE in keeping with ZN/ZNO REDOX REACTIONS; PETER G. LOUTZENHISER, ANTON MEIER, DANIEL GSTOEHL, AND ALDO STEINFELD; four. HYDROTHERMAL CONVERSION OF CO2 INTO VALUE-ADDED items: a possible know-how for making improvements to worldwide CARBON CYCLE; FANGMING JIN, ZHIBAO HUO, XU ZENG, AND HEIJI ENOMOTO; five. ELECTROCATALYTIC relief OF CO2 TO SMALL natural MOLECULE FUELS ON steel CATALYSTS; WENZHEN LI; 6. CO2 CHEMISTRY AT NANKAI workforce: CATALYTIC CONVERSION OF CO2 INTO VALUE-ADDED chemical compounds; LIANG-NIAN HE, ZHEN-ZHEN YANG, AN-HUA LIU, AND JIAN GAO; 7. OXIDATIVE DEHYDROGENATION OF ETHANE TO AND
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Thus, we propose a process for converting CO2 into organics under hydrothermal conditions in the presence of organics or biomass. Scheme 1 shows the rationale of the proposed process. Hydrogen or its species split from water under hydrothermal conditions is used as a reactant to directly reduce CO2 into organics in situ. At the same time, oxygen its species split from water oxidizes organic water or biomass into value-added products. The proposed process has many advantages over water-splitting cycles, including the following: (i) excess oxygen is not required because oxygen is used chemically and (ii) no hydrogen is required, including pumps or storage, because it is derived from water and reacted with CO2 in situ.
Shen. Z. D Thesis, Tongji University, China, 2009, in Chinese. 51. Tenou, S. D Thesis, Tohoku University, Japan, 1997, in Japanese. 52. ; Enomoto, H. Chem. Lett. 2005, 34, 1560–1561. 53. ; Enomoto, H. J. Jpn. Petrol. Inst. 2005, 48, 272–280. 54. ; Enomoto, H. J. Jpn. Petrol. Inst. 2006, 49, 177–185. 55. ; Enomoto, H. Prepr. Pap. - Am. Chem. , Div. Fuel Chem.
The major products are almost identical in the presence and the absence of CO2, primarily featuring straight-chain n-alkanes with more than 9 carbon atoms. These results suggest that CO2 reduction can be achieved and that EPDM can be converted into oils in the hydrothermal treatment of EPDM in the presence of CO2. At present, our results show that CO2 reduction can be achieved using organic waste as a reductant and that organic waste can be simultaneously converted into oils. ; ACS Symposium Series; American Chemical Society: Washington, DC, 2010.